Dine and Moimenta, two of the prettiest villages in the western half of the park, are connected by a high-altitude road with panoramic views of the windmill-speckled hills along the Spanish border. In well-preserved Dine, you can visit a tiny archaeological museum , which documents the 1984 find by a Danish diplomat of Iron Age remains in a nearby cave. The museum is usually locked, but just ask around and someone will rustle up the French-speaking caretaker, Judite, who may also lead you around to the cave itself – pointing out traditional lime kilns and wild-growing medicinal herbs along the way.
Moimenta has a lovely core of granite houses roofed in terracotta, plus a small baroque church – a rare dose of luxury in this austere corner of Portugal. The pretty 7km Calçada loop trail descends from town into the nearby river gorge, following sections of an old stone roadway across a remarkably well-preserved medieval bridge with a single impressive arch.